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Bilitrium is a chemical element that was known to Federation science by the 24th century, a rare crystalline material that, combined with an antimatter converter, could become a powerful energy source. (DS9 episode: "Past Prologue")
During the Tzenkethi War, the crew of the USS Okinawa discovered bilitrium in several planets of the Entelior system and attempted to hide it from the Tzenkethi. (ST - Typhon Pact novel: Rough Beasts of Empire)
The planet Naia VII was rich in bilitrium, among other valuable materials. A Starfleet Corps of Engineers mining operation there in 2368 excavated these, which were vital for Starfleet to rebuild its strength following the Battle of Wolf 359. (TNG - Assimilation² comic: "Issue 2")